CARS spectral profiles are functionally described by the variation of the square of the total third-order, nonlinear susceptibility with the anti-Stokes frequency shift. This inherent, squared susceptibility signal dependence, when weighted by an experiment dependent convolution, produces a CARS spectral profile which is a problem specific to the experiment design.
NiblerJ. W.McDonaldJ. R.HarveyA. B., “Coherent anti-Stokes Raman spectroscopy of gases,” presented at the 5th International Conference on Raman Spectroscopy, Universitat Freiburg, Freiburg, Germany (2–8 September 1976), Paper 8-A-930.
3.
ShaubW. M.NiblerJ. W.HarveyA. B., J. Chem. Phys.67, 1883 (1977).
4.
NiblerJ. W.ShaubW. M.McDonaldJ. R.HarveyA. B., in Vibrational Spectra and Structure, DurigJ. R., Ed. (Elsevier Scientific Publishing Company, New York, 1977), Vol. 6.
5.
MoyaF.DruetS. A. J.TaranJ. P. E., Opt. Commun.13, 169 (1975).
6.
MoyaF.DruetS. A. J.PealatM.TaranJ. P. E., “Flame investigation by coherent anti-Stokes Raman scattering,” Presented at the AIAA 14th Aerospace Sciences Meeting, Washington, DC (26–28 January 1976), Paper 76–29.
7.
RegnierP.TaranJ. P. E., in Laser Raman Gas Diagnostics, LappM.PenneyC. M., Eds. (Plenum Press, New York, 1974), p. 87.
8.
MoyaF.DruetS. A. J.TaranJ. P. E., Rotational Vibration Spectroscopy of Gases by Coherent Anti-Stokes Raman Scattering: Application to Concentration and Temperature Measurements in Laser Spectroscopy, HarocheS.Peboy-PeyroulaJ. C.HanschT. W.HarrisS. E., Eds. (Springer-Verlag, Berlin, 1975).
9.
PealatM.DruetS. A. J.AttalB.TaranJ. P. E., “Temperature and concentration measurements in reactive media by coherent anti-Stokes Raman scattering,” Presented at the 16th International Symposium on Combustion, M.I.T. Cambridge, MA (15–21 August 1976).
10.
For example, see RohW. B., Systems Research Laboratories, Inc., Reports 6948 (1–5), 2800 Indian Ripple Road, Dayton, OH 45440.
DeWittR. N.HarveyA. B.TollesW. M., “Theoretical development of third-order susceptibility as related to coherent anti-Stokes Raman spectroscopy (CARS),” NRL Memorandum Report 3260, Naval Research Laboratory, Washington, DC (April 1976).
14.
ShaubW. M.HarveyA. B.BjorklundG. C., J. Chem. Phys.67, 2547 (1977).
