Abstract
The neutron Time-Of-Flight (n_TOF) facility at the European Laboratory for Particle Physics (CERN) is a pulsed white-spectrum neutron spallation source producing neutrons for two experimental areas: EAR1, located 185 m downstream of the spallation target, and EAR2, located 20 m above the target. The facility is based on a lead target impacted by a high-intensity 20 GeV/
Introduction: The n_TOF facility at CERN
The neutron Time-Of-Flight (n_TOF) facility at the European Laboratory for Particle Physics (CERN) is composed of a spallation neutron source coupled to two neutron flight paths. Neutron energies are deduced from the time of flight between source and detector, hence the name of the facility. The neutron source is driven by a pulsed proton beam extracted from the Proton Synchrotron (PS) machine of the CERN’s accelerator complex. Up to

n_TOF facility layout. A 20 GeV/
The n_TOF facility is an important tool for studies of neutron-induced reactions, especially for radioactive samples. The n_TOF collaboration is composed of 42 member institutions from Europe, India, Japan, Russia, and Australia. The research purposes include the fields of nuclear physics and astrophysics (Big Bang and stellar nucleosynthesis [5,15]), nuclear technologies (nuclear energy production and waste management [1,18]), nuclear medicine (neutron capture therapy) as well as neutron imaging (including the inspection of highly-activated samples [21]).
The relevant features of the neutron source are:
Wide energy range: from thermal to GeV.
Low repetition rate: 1 pulse every 1.2 s (no superposition between neutrons from different proton pulses).
High energy resolution:
High instantaneous neutron flux:
Thanks to these features (especially the very high instantaneous intensity), the facility is well suited to perform high-precision measurements of neutron cross-sections and to study radioactive isotopes with very low cross-sections, or available in only small quantities, or with very high specific activity.
During CERN’s Long Shutdown 2 (LS2), the facility is undergoing an important consolidation and upgrade, which – amongst other activities – includes the construction and installation of the new third-generation spallation target.
Target #1 (2000–2004)
The n_TOF facility was conceived to perform accurate neutron cross-section measurements for different purposes [22]: design of Accelerator Driven Systems (ADS), transmutation of radioactive waste, astrophysics research (synthesis of heavy elements in the Universe), and advancement in fundamental knowledge of nuclear physics.
The facility was commissioned in 2000, with the 185 m horizontal flight path. The first-generation target (Target #1, Fig. 2) was made of a series of pure lead bricks [2], stacked together to form a massive block (

The target was designed to receive 4 pulses of
In 2004, after three years of successful operation, an abnormal increase of radioactivity in the cooling circuit was observed. The issue was ascribed to inefficient cooling at the beam impinging point and lack of chemical control of the cooling water, facilitating pitting corrosion and contamination of water with radioactive lead spallation products [3].
A second-generation target was then designed (Target #2), aimed at addressing the operational concerns of the first-generation target [9]. Target #2 is a cylinder with diameter of 60 cm and axial length of 40 cm, cooled by a forced flow of water (
The target was installed at the end of 2008 and started operation in early 2009. Some critical aspects of the design were highlighted, like the very low thickness (
Another critical aspect was that direct contact between pure lead and cooling water was still present, with the risk of erosion-corrosion phenomena and contamination of the cooling water with radioactive spallation products from lead. Different measures were taken to reduce this risk. The circulation of cooling water was improved, the average beam intensity limited to
Due to these critical aspects, the target was produced and installed considering an estimated lifetime of about ten years. In the last years of target operation, an increase in the cooling water activity was detected and first signs of corrosion of the neutron window were also observed by endoscopic inspection, confirming the necessity of replacing the target with a new one [13].
In 2014 the new experimental area (EAR2) was built 20 m above the target [14]. Even if the design included the possibility of inserting a vacuum tube on top of the spallation target, the resolution in EAR2 was not optimal, since the target shape was not conceived for this experimental area: the moderation of the neutrons directed upwards was achieved with the cooling-water volume above the lead target core, which had an irregular shape.
Target #3: Evolution of the design
The design of the new-generation spallation target (Target #3) began in 2016 with preliminary studies of different target concepts [10].
The objectives to be pursued by the new design were:
Limiting erosion-corrosion phenomena and contamination of the cooling water with lead spallation products.
Improving neutron fluence and resolution for EAR2, thanks to the addition of a dedicated moderator.
Allowing a higher beam pulse intensity to be accepted (from
Preserving the excellent physics performances at EAR1.
Preserving or improving background conditions in the experimental areas.
In the preliminary design stage, six different concepts were evaluated. Based on these studies, two more concepts (for a total of eight) were derived from the preliminary ones, including the final design choice. Figure 3 compares the neutron fluence to EAR1 downstream of the target with respect to Target #2, estimated by FLUKA Monte Carlo code [6,17] for the six preliminary solutions. Figure 4 shows a similar comparison between the three most promising solutions with respect to Target #2. The data in Fig. 3 is extracted right after the target for quicker preliminary simulations, while the data in Fig. 4 is extracted at the EAR1 to show a comparison that is more meaningful for the final decision.
The plot shows the neutron fluence towards the first experimental area (EAR1) right after the target, for the six preliminary design proposals. The neutron fluence has been estimated by means of FLUKA Monte Carlo code [10]. Neutron fluence at EAR1 of the three most promising solutions with respect to Target #2.



The final design of the n_TOF Target #3 is based on six pure lead slices, as shown in Fig. 6. To ensure that lead impurities will have a negligible effect on physics performances, the base lead material has a minimum purity of 99.9 wt%. Shape and size of the slices have been defined after an optimization procedure directed to find the best compromise between the neutron flux towards EAR1 and EAR2, as well as to keep the background low. The slices are 60 cm wide and tall, and 5 cm thick. The only exception is the last slice along the beam direction, which is 15 cm thick to keep the background low. The flat top helps improving the resolution for EAR2 [12].

Exploded view (3D model) of the n_TOF Target #3 final design [12]. Left: cradle assembly. Right: whole target assembly.
The lead slices are cooled down by a forced flow of pure nitrogen. Switching from the water cooling of Target #2 to nitrogen cooling in Target #3 reduced the heat removed per unit area. To keep the same peak temperature in the new target, the surface exposed to the coolant must be increased, hence the slicing. The upgrade to nitrogen cooling avoids water contamination issues, while the absence of cladding materials keeps the background low. In case undesired interactions between nitrogen and lead arise during operation, the cooling system can also work with inert gas (argon) at the cost of a slightly lower cooling efficiency.
This solution is characterized by the best physics performances (neutron flux, background, and resolution) among the ones presented in Section 3 that solve the contamination issues (Fig. 4).
Figure 6 shows the target assembly. The lead slices are supported by an aluminium-alloy structure (Al-6082-T6). This structure has different functions:
supports the lead slices and holds them in place in case of shocks or damage;
regulates the nitrogen flow with cooling channels and constrictions opportunely machined on the aluminum plates;
avoids plastic flow of lead due to creep effects.
The sub-assembly composed of lead slices and aluminum supporting structure is hosted inside a stainless-steel 316L vessel with low cobalt content (around 0.078% with the final batches acquired for production) to reduce the residual dose around the target. The upstream face of the vessel includes a thin window at the beam-impinging location to avoid interaction between proton beam and stainless-steel vessel.
Figure 6 also shows the two moderators, one for each experimental area: the EAR2 moderator is mounted outside of the stainless-steel vessel, above the target, while the EAR1 moderator is integrated into it and represents its downstream face. The two moderator casings are made of aluminum alloy 5083. The bond between the EAR1 moderator and the stainless-steel vessel is realized with a bimetallic transition obtained by a process of explosion cladding. Mechanical tests have been performed on explosion-cladded bonds from different suppliers to validate the solution. The choice of stainless-steel for the vessel instead of aluminum (as in the moderator casings) was requested by the radiation protection team to enhance compatibility with the radioactive wate matrix.
An additional lead plate, shown in Fig. 6 between the stainless-steel vessel and the EAR2 moderator, has been included to reduce the photon background towards EAR2.
The beam parameters representing the worst-case scenario and considered for the design are listed below:
Momentum: 20 GeV/
Protons per pulse:
Energy in one pulse: 32 kJ.
Pulse duration: 6 ns (1
Peak power: 1.8 TW.
Time structure: 6 pulses every 1.2 s followed by 30 s of cool-down, for a supercycle duration totaling 36 s (Fig. 7).
About half of the specified energy and power is absorbed by the target. The target should be able to operate for ten years, until CERN’s Long Shutdown 4 (currently foreseen around 2030). The total number of high intensity pulses impacting the target during its lifetime can be conservatively assumed, for structural fatigue evaluations, equal to
The particle beam impacts the target with a tilt of 10° in the horizontal plane to reduce the EAR1 background caused by
Thermo-mechanical and Computational Fluid Dynamics (CFD) simulations predict the highest temperature to arise in the second lead slice (along the beam direction) and reach 135°C (Fig. 7), safely below the lead melting temperature (327°C) but high enough to provoke reduction in yield strength and creep effects.

Thermal FEM studies of Target #3. Left: peak temperature distribution in the second Pb slice. Right: transients of maximum temperature at periodic regime; the steady-state average is also shown in the plot [12].
The most critical aspect of the target thermo-mechanical response is related to the impulsive character of the thermal load. The quick raise of temperature (over a few nanoseconds), coupled with thermal expansion effects common to all materials, provokes inertia effects, vibrations, and propagation of stress waves. Since the linear-elastic limit stress of pure lead is very low (a few MPa), two kinds of stress wave arise: elastic waves (traveling at the speed of sound in the material) and plastic waves (traveling slower). The details on these thermo-mechanical phenomena and their implications on the target response will be the object of a future publication. The robustness of the lead target when subjected to these phenomena has been tested with a beam irradiation experiment in the CERN’s HiRadMat facility, described in Section 5.
The target will be equipped with mineral-insulated type-K thermocouples to monitor temperature and detect unforeseen changes in the thermal response during operation. The thermocouples will be applied on three points on the surface of the second, third, and sixth lead slice (along the beam direction), close to the spots of highest temperature (the theoretical beam axis). There will be two thermocouples for each of the three points, for a total of six sensors, to have a double measurement for each point. The tip of each thermocouple will be pushed against the lead surface by springs, and their Inconel sheath will be brazed into the stainless-steel feed-through mounted on the external stainless-steel vessel.
A small-scale prototype of Target #3 has been manufactured and tested under beam irradiation in the CERN’s HiRadMat facility [16]. The scope of the facility is the experimental observation of the response of materials when subjected to high-intensity particle-beam pulses. Samples of different materials or prototypes of beam intercepting devices can be temporarily installed in the facility, equipped with different measuring instruments and sensors to measure their response.
The particle beam is supplied by the Super Proton Synchrotron (SPS) ring of the CERN’s accelerator complex, with a momentum of 440 GeV/
The irradiated prototype consists of a series of six lead blocks and is shown in Fig. 8.

Small-scale prototype of the Target #3 final design, tested under beam irradiation in the CERN’s HiRadMat facility.
The second block along the beam direction has a size of
As mentioned in Section 3, a prototype of the Ti-6Al-4V-cladded solution has also been tested. This second prototype consists of a lead cylinder (
The experiment on the first prototype (lead blocks in nitrogen) had the objective of studying, by post irradiation analyses, the effects in the Pb blocks due to repeated beam impacts (presence of voids, defects, etc.) at temperatures between 100 and 140°C. The temperature in each block has been kept steady at the desired values thanks to a series of heating foils applied to the vessel, and monitored by thermocouples applied to each block.
The experiment on the second prototype (Ti-6Al-4V-cladded Pb) had the objective of testing the ability of the Ti-6Al-4V container to resist repeated beam pulses and to measure the dynamic response of the core. The prototype has been impacted by 1000 pulses, each composed of
The lead blocks of the first prototype have been examined by neutron tomography at the Paul Scherrer Institut (PSI) in Switzerland to detect the onset of damage and voids hidden in the bulk of the material. The tomographic examination did not show any material damage. The lead blocks will then be subject to ultrasonic tests and destructive inspections with microstructural examinations.
Once the residual dose rate will be low enough, the second prototype (Ti-6Al-4V-cladded Pb) will also be examined by neutron tomography and destructive inspections: the core will be extracted from the water vessel and the bulk of the lead cylinder will be inspected to detect damage in the material and changes in microstructure.
After three years of design and R&D activities, many possible solutions evaluated, and four project reviews, the third-generation neutron spallation target for the n_TOF facility at CERN is entering in the production stage in 2019. The design studies led to a target concept based on 99.9+ wt% pure lead blocks, supported by an aluminum 6082-T6 structure and cooled by gaseous nitrogen. The assembly will be enclosed in a stainless-steel 316L vessel and equipped with water moderators with aluminum 5083 casings, one for each experimental area. The temperature of the target’s lead core will be monitored by opportunely mounted thermocouples. All the critical aspects of the design, like the explosion-bonded bimetallic transition joining the stainless-steel 316L vessel to the aluminum 5083 moderator casing, have been prototyped, tested, and validated. The dynamic response of the target core, when impacted by high-intensity proton-beam pulses, has been studied and tested in a beam-irradiation experiment in the CERN’s HiRadMat facility, both for the baseline design concept and for an alternative titanium-cladded solution of the target core.
The production of the target will continue during 2020. The installation of the target is planned for the same year, and commissioning with beam will take place in 2021.
Future publications on the detailed thermo-mechanical studies performed on the target are planned. The aspects of main scientific interest include:
the high-strain rate response of the lead core subjected to impulsive thermal load and its implementation in numerical models;
the low-strain rate plastic flow of the lead core due to creep effects and its implementation in numerical models;
the preparation of the beam irradiation tests, the experimental results and their correlation with numerical models.
