Abstract
The kinetics of reaction of collagen peptide with allyl glycidyl ether (AGE), and their temperature dependence, were studied by monitoring the reduction of the primary amine groups as a function of time. A kinetic model, with a second order with respect to the primary amine groups of collagen peptide and a first-order dependence on AGE, was developed that gave a good fit to the experimental data.
References
1.
Gantar A.
,
Šebenik A.
,
Kavčič M.
,
Osredkar U.
, and
Harwood H. J.
(1987 ) Polymer , 28 , 1403 .
2.
Tu R.
,
Lu C.-L.
,
Thyagarajan K.
,
Wang E.
,
Nguyen H.
,
Shen S.
,
Hata C.
, and
Quijano R. C.
(1993 ) J. Biomed. Mater. Res. , 27 , 3 .
3.
Sung H. W.
,
Hsu C. S.
,
Lee Y. S.
, and
Lin D. S.
(1996 ) J. Biomed. Mater. Res. , 31 , 511 .
4.
Zeeman R.
,
Dijkstra P. J.
,
van Wachem P. B.
,
van Luyn M. J. A.
,
Hendriks M.
,
Cahalan P. T.
, and
Feijen J.
(2000 ) J. Biomed. Mater. Res. , 51 , 541 .
5.
Nagura M.
,
Yokota H.
,
Ikeura M.
, and
Gotoh Y.
(2002 ) Polym. J. , 34 , 761 .
6.
Kaul G.
,
Lee-Parsons C.
, and
Amiji M.
(2003 ) Pharm. Eng. , 23 , 1 .
7.
Gratzer P. F.
,
Santerrec J. P.
, and
Lee J. M.
(2004 ) Biomater. , 25 , 2081 .
8.
Di Y.
,
Heath R. J.
,
Long A.
, and
Hartnung K.
(2006 ) J. Soc. Leather Technol. Chem. , 90 , 93 .
9.
Pšeja J.
,
Hmčiřìk J.
,
Rupee J.
,
Charvátová H.
,
Hruzík P.
, and
Tupý M.
(2006 ) J. Polym. Environ. , 14 , 231 .
10.
Kurniawan L.
,
Qiao G. G.
, and
Zhang X. Q.
(2007 ) Biomacromolecules , 8 , 2909 .
11.
Vargas G.
,
Acevedo J. L.
,
Lopez J.
, and
Romero J.
(2008 ) Mater. Lett. , 62 , 3658 .
12.
Fraenkel-Conrat H.
(1944 ) J. Biol. Chem. , 154 , 227 .
13.
Sung H. W.
,
Chen W. H.
,
Chiu I. S.
,
Hsu H. L.
, and
Liu S. A.
(1996 ) J. Biomed. Mater. Res. , 33 , 177 .
14.
Eloundou J. P.
,
Feve M.
,
Harran D.
, and
Pascault J. P.
(1995 ) Macromol. Mater. Eng. , 230 , 13 .
15.
Jiang T. D.
(2006 ) Collagen and gelatin , Chemical Industry Press , Beijing .
16.
Wu L. Y.
,
Zheng Y. T.
,
Wu Y.
, and
Shang Z. F.
(2008 ) Chemistry (Peking) , 71 , 158 .
17.
Ward A. G.
(1977 ) The science and technology of gelatin , Academic Press , New York .
18.
Zhang L. X.
(1981 ) Laboratory methods and techniques in biological chemistry , Peoples Education Press , Beijing .
19.
Wright Y
,
McGarraugh G.
, and
Phillips R.
(1980 ) Polymer , 21 , 1167 .
20.
Tu R.
,
Lu C.-L.
,
Thyagarajan K.
,
Wang E.
,
Nguyen H.
, and
Quijano R. C.
(1991 ) ASAIO Meeting , Chicago, Illinois , April 25–27.
21.
Morrison R. T.
, and
Boyd R. N.
(1986 ) Organic chemistry , 4th edn, Allyn and Bacon , Boston .
22.
Enikolopiyan N. S.
(1976 ) Pure Appl. Chem. , 48 , 317 .
23.
Flammersheim H. J.
(1998 ) Thermochim. Acta , 310 , 153 .