Polycyclic aromatic hydrocarbons (PAHs) are a kind of carcinogenic, teratogenic and mutagenic pollutants that exist widely. In this study, a quarterly emission inventory of 16 PAHs listed as the US EPA priority pollutants was established by using the emission factor (EF) method. The results showed that the distribution of PAHs in different industries varied greatly with different year and quarter. The main characteristics of PAHs seasonal emission are that Q1 emission is the most and Q4 emission is the least. Among them, naphthalene and phenanthrene are the most important compounds. There are significant differences in PAHs emissions from different sources. Traffic and civil use emissions are the main sources. For example, in 2019, traffic emissions accounted for 20.9% and civil use emissions accounted for 78.3% of the total emissions. Then, a linear multiple regression model was established to predict the quarterly emission of PAHs. A vector autoregressive (VAR) approach was applied to analyse the correlation between the gross domestic product (GDP) and other macroeconomic parameters. This study could be used as a guide to provide recommendations for government policy and macro-control efforts.
LiJYuanGLLiPSunYYuHHWangGH.The emerging source of polycyclic aromatic hydrocarbons from mining in the Tibetan Plateau: distributions and contributions in background soils. Sci Total Environ2017; 584: 64–71.
2.
HamidNSyedJHJunaidMMahmoodALiJZhangGMalikRN.Elucidating the urban levels, sources and health risks of polycyclic aromatic hydrocarbons (PAHs) in Pakistan: implications for changing energy demand. Sci Total Environ2018; 619: 165–175.
3.
FangYChenYJHuLMTianCGLuoYMLiJZhangGZhengMLinT.Large-river dominated black carbon flux and budget: a case study of the estuarine-inner shelf of East China Sea, China. Sci Total Environ2019; 651: 2489–2496.
4.
BlasingMAmelungWSchwarkLLehndorffE.Inland navigation: PAH inventories in soil and vegetation after EU fuel regulation 2009/30/EC. Sci Total Environ2017; 584: 19–28.
5.
JungKHKimJKNohJHEunJWBaeHJKimMGChangYGShenQKimSJKwonSHParkWSLeeJYNamSW.Characteristic molecular signature for the early detection and prediction of polycyclic aromatic hydrocarbons in rat liver. Toxicol Lett2013; 216: 1–8.
6.
DiggsDLHudersonACHarrisKLMyersJNBanksLDRekhadeviPVNiazMSRameshA.Polycyclic aromatic hydrocarbons and digestive tract cancers: a perspective. J Environ Sci Health C Environ Carcinog Ecotoxicol Rev2011; 29: 324–357.
ChaoCYHYeungLLChoiPSH.Quantification of polycyclic aromatic hydrocarbons and aliphatic hydrocarbons in air particulate samples in homes. Indoor Built Environ2002; 11: 123–133.
9.
MadanyICrumpDR.The burning of incense as an indoor source of volatile organic compounds. Indoor Built Environ1994; 3: 292–298.
10.
CuleaMCozarOCuleaE.PAHs in cigarette smoke by gas chromatography-mass spectrometry. Indoor Built Environ2005; 14: 283–292.
11.
SugiyamaTAmagaiTMatsushitaHSomaM.Size distribution of polycyclic aromatic hydrocarbons in indoor airborne particulates. Indoor Built Environ2000; 9: 265–276.
12.
ShenHHuangYWangRZhuDLiWShenGWangBZhangYChenYLuYChenHLiTSunKLiBLiuWLiuJTaoS.Global atmospheric emissions of polycyclic aromatic hydrocarbons from 1960 to 2008 and future predictions. Environ Sci Technol2013; 47: 6415–6424.
13.
ZhangYTaoS.Seasonal variation of polycyclic aromatic hydrocarbons (PAHs) emissions in China. Environ Pollut2008; 156: 657–663.
14.
ZhangYXTaoS.Global atmospheric emission inventory of polycyclic aromatic hydrocarbons (PAHs) for 2004. Atmos Environ2009; 43: 812–819.
15.
ZhangYL.Dynamic effect analysis of meteorological conditions on air pollution: A case study from Beijing. Sci Total Environ2019; 684: 178–185.
16.
XuXZ.Study on the relationship between the economic growth and environmental pollution in Fujian province based on the VAR model. Boca Raton, FL: CRC Press – Taylor & Francis Group, 2015, pp.333–337.
17.
KumarUPrakashAJainVK.A multivariate time series approach to study the interdependence among O-3, NO (x) and VOCs in ambient urban atmosphere. Environ Model Assess2009; 14: 631–643.
18.
TianHZhaoDWangY.Emission inventory of air pollutants from biomass combustion in China. J Environ Sci2011; 31: 349–357.
19.
ZuoQDuanYHYangYWangXJTaoS.Source apportionment of polycyclic aromatic hydrocarbons in surface soil in Tianjin, China. Environ Pollut2007; 147: 303–310.
20.
ZhangHFHuDWChenJMYeXNWangSXHaoJMWangLZhangRYAnZS.Particle size distribution and polycyclic aromatic hydrocarbons emissions from agricultural crop residue burning. Environ Sci Technol2011; 45: 5477–5482.
21.
MuX.Emission inventory of polycyclic aromatic hydrocarbons in China. MA Thesis, China University of Petroleum, Beijing, 2016. (in Chinese)
22.
YangCSuHChengYHuangYLiuWSHenGDUanYLiuWTaoS.Emission characteristics of particulate matter and polycyclic aromatic hydrocarbons from firewood and honeycomb coal in rural areas of Taigu, Shanxi Province. J Ecotoxicol2014; 9: 545–555. (in Chinese)
23.
HanDBiaoCWeiZQiuWLiuSLiuYLiuWTaoS.Study on emission factors of polycyclic aromatic hydrocarbons in domestic civil coal-fired flue gas. J Environ Sci2007; 27: 1783–1788.
24.
China NBosotpsRo. National Bureau of statistics of the People's Republic of China, https://data.stats.gov.cn/index.htm (2020, accessed 20 December 2020).
PeterKTTianZYWuCLinPWhiteSDuBWMcIntyreJKScholzNLKolodziejEP.Using high-resolution mass spectrometry to identify organic contaminants linked to urban stormwater mortality syndrome in Coho Salmon. Environ Sci Technol2018; 52: 10317–10327.
WangT.Study on vehicle emission inventory of Chongqing urban area based on IVE model (in Chinese). J Chongqing Jiaotong Univ (Natural Science Edition)2014; 33: 135–137.
29.
HeXZhangXWuYLvJ.Analysis of vehicle mileage distribution by annual inspection data.Light Industry Technol2017; 000: 87–89. (in Chinese)
30.
AgrawalHSawantAAJansenKMillerJWCockerDR.Characterization of chemical and particulate emissions from aircraft engines. Atmos Environ2008; 42: 4380–4392.
31.
Al-DhurafiNAMasseranNZamzuriZH.Compositional time series analysis for Air Pollution Index data. Stoch Environ Res Risk Assess2018; 32: 2903–2911.
PesaranMHShinY.Impulse response analysis in linear multivariate models. Econom Lett1998; 58: 17–29.
34.
ZhangYDouHChangBWeiZQiuWLiuSLiuWTaoS.Emission of polycyclic aromatic hydrocarbons from indoor straw burning and emission inventory updating in China. Ann N Y Acad Sci2008; 1140: 218–227.
35.
NiuLZhouYXuCZhangCZhouJZhangXLiuW.Solid fuel combustion as a major contributor of polycyclic aromatic hydrocarbons in rural China: evidence from emission inventory and congener profiles in tree bark. Environ Pollut2019; 246: 621–629.
36.
LiXPengLYaoXJCuiSLHuYYouCZChiTH.Long short-term memory neural network for air pollutant concentration predictions: Method development and evaluation. Environ Pollut2017; 231: 997–1004.
37.
BaiLLiCYuCWHeZ.Air pollution and health risk assessment in northeastern China: a case study of Jilin Province. Indoor Built Environ, epub ahead of print 21 January 2021, https://doi.org/10.1177/1420326X20979274.
WangH-Y.Analysis of the sustainable development strategy of the China highway policy. J Highway Transp Res Dev (English Ed)2016; 10: 103–110.
41.
YuanXLLiuXZuoJ.The development of new energy vehicles for a sustainable future: a review. Renew Sustain Energy Rev2015; 42: 298–305.
42.
ZhangXBaiX.Incentive policies from 2006 to 2016 and new energy vehicle adoption in 2010-2020 in China. Renew Sustain Energy Rev2017; 70: 24–43.
43.
EmbialeAZewgeFChandravanshiBSSahle-DemessieE.Short-term exposure assessment to particulate matter and total volatile organic compounds in indoor air during cooking Ethiopian sauces (Wot) using electricity, kerosene and charcoal fuels. Indoor Built Environ2019; 28: 1140–1154.
MaWLLiYFQiHSunDZLiuLYWangDG.Seasonal variations of sources of polycyclic aromatic hydrocarbons (PAHs) to a northeastern urban city, China. Chemosphere2010; 79: 441–447.
47.
HeJFanSMengQSunYZhangJZuF.Polycyclic aromatic hydrocarbons (PAHs) associated with fine particulate matters in Nanjing, China: distributions, sources and meteorological influences. Atmos Environ2014; 89: 207–215.
48.
YishenZHouyongZShengjiLLiWuZLingyanHXiaofenHJianshenW.Emission characteristics of PAHs fromopenand residential biomassburning. China Environ Sci2015; 35: 387–395.
49.
Ray-MukherjeeJNimonKMukherjeeSMorrisDWHamerM.Using commonality analysis in multiple regressions: a tool to decompose regression effects in the face of multicollinearity. Methods Ecol Evol2014; 5: 320–328.
50.
UekiMKawasakiYJCSAnalysisD.Multiple choice from competing regression models under multicollinearity based on standardized update. Computat Stat Data Analys2013; 63: 31–41.
51.
JohansenSRJuseliusK.Maximum likelihood estimation and inference on cointegration – with applications to the demand for money. Oxford Bull Econom Stats2010; 52: 169–210.
52.
LiZLSunLGengYDongHJRenJZLiuZTianXYabarHHiganoY.Examining industrial structure changes and corresponding carbon emission reduction effect by combining input-output analysis and social network analysis: a comparison study of China and Japan. J Cleaner Product2017; 162: 61–70.
53.
Yi-Jun Y Rong-HuiX.Research on the effect of environmental regulation to industrial restructuring-empirical test based on provincial panel data of China. China Acad J2014; 8: 57–69.
54.
RenSGYuanBLMaXChenXH.International trade, FDI (foreign direct investment) and embodied CO2 emissions: a case study of Chinas industrial sectors. China Econom Rev2014; 28: 123–134.
55.
HongyanWFeiWRenhuaSChunyuGYajingWNingSLeiWYuyunB.Review of foreign policies and regulations on crop straw utilization and its experience and enlightenment.J Agricultural Eng2016; 32: 216–222. (in Chinese)
56.
NanakiEAXydisGAKoroneosC.Electric vehicle deployment in urban areas. Indoor Built Environ2016; 25: 1065–1074.
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