Thermomechanical viscoelastic response of a unidirectional graphite/polyimide composite at elevated temperatures using a micromechanical approach

Abstract

In this work, the thermomechanical viscoelastic response of a high temperature polymer matrix composite system made up of T650-35 graphite fibers embedded in PMR-15 resin is studied through a micromechanical model based on the assumptions of simplified unit cell method within a temperature range of 250–300℃ corresponding to aerospace engine applications. The advantage of this particular micromechanical model lies in its ability to give closed-form expressions for the effective viscoelastic response of unidirectional composites as well as each of their constituents. Using the experimental data of the creep behavior of thermostable PMR-15 polyimide, the micromechanical model is first calibrated to account for the effect of temperature. The resulting elastic and viscoelastic responses are found to be in good agreement with the existing experimental data. The validated model is then used to predict the behavior of the composite material under different combinations of thermal and mechanical loadings. The results clearly demonstrate the importance of accounting for the viscoelastic effect of the matrix material as the temperature increases. Current works on modeling temperature-dependent viscoelastic behavior of polymer matrix composites are mainly based on the assumption of thermorheologically simple material. However, through the present approach where the matrix is modeled as a thermorheologically complex material, the effect of temperature on the elastic and viscoelastic response of the composite system can be individually investigated.